The three traitorous Students Kenji Tsukigata, Rui Senda and Gou Omura come back from Outer Space in the name of the Armed Brain Army Volt to begin their attack on the Earth.
Daisuke Shima
Yusuke Amamiya / Red Falcon
Kazuhiko Nishimura
Jo Oohara / Yellow Lion
Megumi Mori
Megumi Misaki / Blue Dolphin
Seiro Yamaguchi
Tetsuya Yano / Black Bison
Jin Kawamoto
Jun'ichi Aikawa / Green Sai
Makoto Kousaka
Colon (voice)
Jouji Nakata
Great Professor Bias
Yutaka Hirose
Kenji Tsukigata / Doctor Kemp
Akiko Amamatsuri
Rui Senda / Doctor Mazenda
Toru Sakai
Goh Omura / Doctor Obler
Takeshi Kuwabara
Narrator
Daisuke Ban
Doctor Hoshi
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